This paper describes Century Soil Organic Matter (SOM) Model simulations of seven long-term data sets that are the subject of this special issue. We found that Century successfully simulates SOM C across a variety of land use and climate types. Simulations of SOM were most successful in grass and crop systems. This exercise highlights a structural limitation of Century in simulating SOM in a forest with a developed litter layer. Simulations of tree biomass distributions, however, were generally successful. The model failed to capture extreme values of yield and N offtake, although annual averages were quite similar between observations and simulations, leading to reasonable estimates of SOM C. Average yields and SOM were generally higher in amended treatments or rotations including an N-fixing component such as alfalfa. The model successfully predicted SOM dynamics across climates, land use types, and treatments. This suggests that Century is a useful tool for ecosystem studies, particularly those focused on SOM dynamics. (C) 1997 Elsevier Science B.V.